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Electronic Excitations at Metal Surfaces

Electronic Excitations at Metal Surfaces PDF Author: Ansgar Liebsch
Publisher: Springer Science & Business Media
ISBN: 1475751079
Category : Science
Languages : en
Pages : 347

Book Description
In this new work, the focus is on the dynamical response of metal electrons to several types of incident electromagnetic fields. The author, an eminent theorist, discusses Time-Dependent Local Density Approximation's importance in both elucidating electronic surface excitations and describing the ground state properties of electronic systems. Chapters detail theoretical formulations and computational procedures, covering such areas as single-particle and collective modes, spatial distribution of the induced surface charges, and local electric fields. Excitation spectra are shown for a variety of clean simple metals, noble metals, chemisorbed overlayers, charged surfaces, and small metal particles.

Electronic Excitations at Metal Surfaces

Electronic Excitations at Metal Surfaces PDF Author: Ansgar Liebsch
Publisher: Springer Science & Business Media
ISBN: 1475751079
Category : Science
Languages : en
Pages : 347

Book Description
In this new work, the focus is on the dynamical response of metal electrons to several types of incident electromagnetic fields. The author, an eminent theorist, discusses Time-Dependent Local Density Approximation's importance in both elucidating electronic surface excitations and describing the ground state properties of electronic systems. Chapters detail theoretical formulations and computational procedures, covering such areas as single-particle and collective modes, spatial distribution of the induced surface charges, and local electric fields. Excitation spectra are shown for a variety of clean simple metals, noble metals, chemisorbed overlayers, charged surfaces, and small metal particles.

Ab Initio Theory of Electronic Excitations at Surfaces

Ab Initio Theory of Electronic Excitations at Surfaces PDF Author: Matthias Timmer
Publisher: Sudwestdeutscher Verlag Fur Hochschulschriften AG
ISBN: 9783838122694
Category :
Languages : en
Pages : 172

Book Description
Understanding energy dissipation mechanisms is a field of present-day scientific interest. Experimental results for electronic excitations in metals propose a measurable electronic excitation during many processes involving a metal surface, including epitaxy. While the role of the nuclear excitation processes is comparatively well understood, the role of electronic excitation processes in the energy dissipation during adsorption and other dynamical processes at surfaces is elusive. One of the reasons is that the interaction dynamics is often treated on a Born- Oppenheimer potential energy surface, which is, strictly speaking, not justified for metals, but lifting this restriction is computationally demanding. The focus of this book is the investigation of a perturbative approach to calculate electronic excitations. After a basic introduction into some major aspects of Density Functional Theory calculations, a time-dependent perturbative approach to calculate electronic excitations is developed. This approach is then applied to several model systems, and the results are compared to available experimental data, and other theoretical approaches.

Theoretical Surface Science

Theoretical Surface Science PDF Author: Axel Groß
Publisher: Springer Science & Business Media
ISBN: 3540689699
Category : Technology & Engineering
Languages : en
Pages : 342

Book Description
Progress continues in the theoretical treatment of surfaces and processes on surfaces based on first-principles methods, i.e. without invoking any empirical parameters. In this book, the theoretical concepts and computational tools necessary and relevant for a microscopic approach to the theoretical description of surface science is presented, together with a detailed discussion of surface phenomena. This makes the book suitable for both graduate students and for experimentalists seeking an overview of the theoretical concepts in surface science. This second enlarged edition has been carefully revised and updated, a new chapter on surface magnetism is included, and novel developments in theoretical surface science are addressed.

Laser Spectroscopy and Photochemistry on Metal Surfaces

Laser Spectroscopy and Photochemistry on Metal Surfaces PDF Author: Hai-Lung Dai
Publisher: World Scientific Publishing Company Incorporated
ISBN: 9789810229993
Category : Science
Languages : en
Pages : 1420

Book Description
III. Desorption dynamics. 16. Electromically stimulated desorption of neutrals and ions from adsorbed and condensed layers / P. Feulner and D. Menzel -- 17. State-resolved probes of molecular desorption dynamics induced by short-lived electronic excitations / E. Hasselbrink -- 18. Laser-induced desorption / Yoshitada Murata and Katsuyuki Fukutani -- 19. Femtosecond surface science: the dynamics of desorption / J.A. Misewich ... [et al.] -- 20. Femtosecond probing of chemical reaction dynamics at surfaces / Harry W.K. Tom and Judith A. Prybyla -- 21. Hot electrons and photodesorption dynamics: theory / J.W. Gadzuk -- 22. Electronic dynamics of chemisorbed molecules: an adiabatic model of photodesorption and spectroscopy / D.R. Jennison, E.B. Stechel, and A.R. Burns -- 23. Hydrogen recombinative desorption dynamics / Stacey F. Bent, Hope A. Michelsen, and Richard N. Zare -- IV. Photochemistry. 24. Surface photochemistry / W. Ho -- 25. Photodissociation and photoreaction of molecules attached to metal surfaces / X.L. Zhou and J.M. White -- 26. Dynamics of adsorbate photochemistry / J.C. Polanyi and Y. Zeiri -- 27. Adsorbate photochemical dynamics on Pt (111) / I. Harrison -- 28. Photochemistry at low temperatures / René Franchy -- 29. Laser-induced polymerization on surfaces / Z.C. Ying, L.E. Fleck, and H.-L. Dai

Photonic Probes of Surfaces

Photonic Probes of Surfaces PDF Author: P. Halevi
Publisher: Newnes
ISBN: 0444599347
Category : Technology & Engineering
Languages : en
Pages : 588

Book Description
This volume is devoted principally to optical spectroscopies of material surfaces and also encompasses scattering techniques and theoretical response analysis as well as spectroscopies. In addition to solid surfaces some attention is also devoted to interfaces between two solids, between a solid and a liquid and to a liquid-vapor interface. These surfaces may be clean and perfect, in which case the purpose of the spectroscopical method at hand is to determine the deviation of the atomic structure in the surface region from that in the bulk, namely the surface reconstruction. Otherwise the surface may be imperfect due to roughness, strain or overlayers, in which case the spectroscopy can yield information on the nature of such imperfections, including the monitoring of growth processes. One of the foremost purposes of surface spectroscopies is to extract information on atomic and molecular adsorbates on solid surfaces. Most of the 10 chapters are concerned with photonic sources of excitation, the respective spectral regions ranging from the far infrared to X-rays. In conclusion this book provides a state-of-the-art review of all major types of photonic probes of surfaces and interfaces and deals with both applications and experiment and theory.

Materials Modification by Electronic Excitation

Materials Modification by Electronic Excitation PDF Author: Noriaki Itoh
Publisher: Cambridge University Press
ISBN: 9780521554985
Category : Science
Languages : en
Pages : 658

Book Description
Electronic excitation is a means to change materials properties. This book analyses the important features of the changes induced by electronic excitation, identifies what is critical, and provides a basis from which materials modification can be developed successfully. Electronic excitation by lasers or electron beams can change the properties of materials. In the last few years, there has been a mix of basic science, of new laser and electron beam tools, and of new needs from microelectronics, photonics and nanotechnology. This book extends and synthesises the science, addressing ideas like energy localisation and charge localisation, with detailed comparisons of experiment and theory. It also identifies the ways this understanding links to technological needs, like selective removal of material, controlled changes, altering the balance between process steps, and possibilities of quantum control. This book will be of particular interest to research workers in physics, chemistry, electronic engineering and materials science.

Laser Spectroscopy and Photochemistry on Metal Surfaces

Laser Spectroscopy and Photochemistry on Metal Surfaces PDF Author: Hai-Lung Dai
Publisher: World Scientific
ISBN: 981431725X
Category : Science
Languages : en
Pages : 819

Book Description
Using lasers to induce and probe surface processes has the advantages of quantum state specificity, species selectivity, surface sensitivity, fast time-resolution, high frequency resolution, and accessibility to full pressure ranges. These advantages make it highly desirable to use light to induce, control, or monitor surface chemical and physical processes. Recent applications of laser based techniques in studying surface processes have stimulated new developments and enabled the understanding of fundamental problems in energy transfer and reactions. This volume will include discussions on spectroscopic techniques, energy transfer, desorption dynamics, and photochemistry.

Laser Spectroscopy and Photochemistry on Metal Surfaces

Laser Spectroscopy and Photochemistry on Metal Surfaces PDF Author: H-L Dai
Publisher: World Scientific
ISBN: 981450209X
Category : Technology & Engineering
Languages : en
Pages : 1464

Book Description
0Keywords:Surface Photochemistry;Photochemistry;Laser Spectroscopy;Surface Spectroscopy;Photodesorption;Surface Dynamics;Surface Femtochemistry;Surface Nonlinear Optics;Surface Analysis;Metal Surfaces

Dynamics at Solid State Surfaces and Interfaces, Volume 1

Dynamics at Solid State Surfaces and Interfaces, Volume 1 PDF Author: Uwe Bovensiepen
Publisher: Wiley-VCH
ISBN: 9783527409372
Category : Science
Languages : en
Pages : 0

Book Description
This two-volume work covers ultrafast structural and electronic dynamics of elementary processes at solid surfaces and interfaces, presenting the current status of photoinduced processes. Providing valuable introductory information for newcomers to this booming field of research, it investigates concepts and experiments, femtosecond and attosecond time-resolved methods, as well as frequency domain techniques. The whole is rounded off by a look at future developments.

Reviews in Plasmonics 2010

Reviews in Plasmonics 2010 PDF Author: Chris D. Geddes
Publisher: Springer Science & Business Media
ISBN: 1461408849
Category : Medical
Languages : en
Pages : 338

Book Description
Reviews in Plasmonics 2010, the first volume of the new book serial from Springer, serves as a comprehensive collection of current trends and emerging hot topics in the field of Plasmonics and closely related disciplines. It summarizes the year’s progress in surface plasmon phenomena and its applications, with authoritative analytical reviews specialized enough to be attractive to professional researchers, yet also appealing to the wider audience of scientists in related disciplines of Plasmonics. Reviews in Plasmonics offers an essential reference material for any lab working in the Plasmonics field and related areas. All academics, bench scientists, and industry professionals wishing to take advantage of the latest and greatest in the continuously emerging field of Plasmonics will find it an invaluable resource. Key features: Accessible utility in a single volume reference. Chapters authored by known leading figures in the Plasmonics field. New volume publishes annually. Comprehensive coverage of the year's hottest and emerging topics. Reviews in Plasmonics 2011 topics include: Metal Nanoparticles for Molecular Plasmonics. Surface Plasmon Resonance based Fiber Optic Sensors. Elastic Light Scattering of Biopolymer/Gold Nanoparticles Fractal Aggregates. Influence of electron quantum confinement on the electronic response of metal/metal interfaces. Melting Transitions of DNA-Capped Gold Nanoparticle Assemblies. Nanomaterial Based Long Range Optical Ruler for Monitoring Biomolecular Activities. Plasmonic Gold and Silver Films: Selective Enhancement of Chromophore Raman Scattering or Plasmon-Assisted Fluorescence.